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259 successfully engineered several artificial photocatalytic cross-coupling enzyme variants by incorporating an Ir photocatalyst via cysteine-maleimide conjugation and a bipyridine nickel Ni II (bpy) in close proximity, the resulting enzyme harnessed visible light to execute intramolecular electron transfer between the two catalysts, leading to C–O coupling products with exceptional yields of up to 96% (Figure 10b)